He was interviewed for the documentary United We Stand, Divided We Fall: The Making of Captain America: Civil War.
- He was nominated for a Saturn Award for Best Supporting Actor for his work on Avengers: Age of Ultron.
- Together with Robert Downey, Jr., Scarlett Johansson, Don Cheadle and Chadwick Boseman, he was nominated for a Teen Choice Award for Choice Movie: Chemistry for his work on Captain America: Civil War.
- Paul Bettany is the husband of Jennifer Connelly. Their son Stellan is named after Stellan Skarsgård.
- Paul Bettany is the first actor to portray two major characters in the Marvel Cinematic Universe.
- Paul Bettany also portrayed Priest in the comic book adaptation Priest.
- Paul Bettany previously worked with Jon Favreau in Wimbledon.
- Paul Bettany worked again with Anthony Mackie in Shelter.
- Paul Bettany admitted in an interview with Digital Spy in 2012 that he had a general disinterest in the Marvel Cinematic Universe and had not seen any of the films until he was cast as Vision, stating that his role as J.A.R.V.I.S. was mainly for financial gain.
- Paul Bettany is one of the actors to portray characters for both Marvel Studios and Lucasfilm, both of which are owned by Walt Disney Pictures. He will star in an untitled Han Solo movie.
- Paul Bettany previously worked with Gwyneth Paltrow in Mortdecai.