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Since this wiki doesn't seem to say "This character is the main antagonist of this film" I'll say it for those who haven't seen them but want to know (though Iron Man 3 is a spoiler):
- Iron Man - Obadiah Stane
- The Incredible Hulk - Abomination
- Iron Man 2 - Ivan Vanko, Justin Hammer
- Thor - Loki
- Captain America: The First Avenger - Red Skull
- The Avengers - Loki
- Iron Man 3 - Aldrich Killian
- Thor: The Dark World - Malekith
- Captain America: The Winter Soldier - Alexander Pierce
- Guardians of the Galaxy - Ronan the Accuser
- Avengers: Age of Ultron - Ultron
- Ant-Man - Darren Cross
- Captain America: Civil War - Helmut Zemo
- Doctor Strange - ???
- Guardians of the Galaxy 2 - ???
- Thor Ragnarok - ???
- Black Panther - ???
- Avengers: Infinity War Part 1 - Thanos
- Captain Marvel - ???
- Inhumans - ???
- Avengers: Infinity War Part 2 - Thanos